Adam West Bruce Wayne / Batman (voice) Burt Ward Dick Grayson / Robin (voice) William Shatner Harvey Dent / Two-Face (voice) Julie Newmar Catwoman (voice) Jeff Bergman Joker / Bookworm / Desmond Dumas (voice) Sirena Irwin Harleen Quinzel (voice) Thomas Lennon Chief O'Hara (voice) Lee Meriwether Lucilee Diamond (voice) William Salyers Penguin (voice) Lynne Marie Stewart Aunt Harriet (voice) Jim Ward Commissioner Gordon / Hugo Strange (voice) Steven Weber Alfred Pennyworth (voice) Wally Wingert Riddler / King Tut (voice) Maurice LaMarche Egghead (voice)